The Third, though wishing to pass the name of Hokage to his favorite student, could not bring himself to knowingly satisfy Orochimaru's lust for power, and thus gave the position to someone else.
Orochimaru, however, craved more power than could be obtained from training with his master, and began abducting villagers of Konohagakure for experimentation. He simultaneously applied for the title of Hokage, the village's protector, hoping that the position would give him access to new abilities.
Orochimaru already died, killed by sasuke and jiraiya by pein (aka leader of akatsuki). Now tsunade only sannin alive. This is sad for me.
Orochimaru Gaiden
No longer having a reason to keep face in Konoha, Orochimaru was less discreet about his abductions and experimentations, giving in the Third the opportunity to discover what he was doing. Unwilling to bring himself to harm Orochimaru, the Third allowed him to escape and flee the village. After the Third uncovered the truth, Orochimaru left Konoha and formed the Hidden Sound Village in the Land of Rice. He was responsible for countless immoral experiments and collected many ninja with unique abilities in his numerous hidden bases. He wished more than anything to find the ultimate body and improve himself to the state of a god.
Personality
Orochimaru's various human experiments take place so as to serve two purposes, most prominent of which is his desire to learn every jutsu in the Naruto world. Jiraiya speculates that this is due to the fact that his parents died when he was at a very young age, and flashbacks shown during his battle with the Third Hokage speak to this effect.
Because a human's lifespan does not allow enough time to learn every jutsu, Orochimaru also experiments on others so as to achieve immortality. By living throughout the ages, Orochimaru need never worry about death and thus all the knowledge he gains will never be lost.
Orochmaru can summoning giant snake called manda, he called him when fight again tsunade and jiraiya.
Fight with the Four Tailed Naruto
After antagonizing Naruto to the point where he transforms into a four-tailed state and attacks him, Orochimaru demonstrates a number of new abilities. As well as modified forms of snake summonings, he can shed his skin like a snake and, by doing so, repair any damage to his body, extend small snakes on his hands that can shoot powerful fire blasts, and absorb the strength of attacks thrown at him strengthening his body with the Soft Physique Modification Jutsu. He also demonstrates his immense reserves of chakra when he summons three Rashomon gates to block the Four-Tailed Strong Ball that the four tailed Naruto's spat at him. Though they failed to block the attack in any way, it was still an impressive feat. Additionally, Orochimaru can create a Battle Clone out of snakes that can morph various parts of its body into snake parts. If injured, it can simply regenerate, and can be controlled from long distances by Orochimaru.
After Sasuke's defection, he spent the next two and half years training the boy to be his next body. When Team Yamato attempted to infiltrate his base for Sasuke, he reappears during a meeting between Yamato, disguised as Sasori, and Kabuto. Orochimaru explains that he had long ago undone Sasori's "Binding Jutsu" on Kabuto, and had intended assassinating his former Akatsuki Partner but never did. He then calls out Naruto, Sakura, and Sai to do battle. He explains that Yamato was the only one out of sixty test subjects that survived one of his genetic experiments to duplicate the First Hokage's Mokuton techniques and his previously unknown ability to "control tailed beasts", though he himself did not recognize this until Yamato revealed the abilities himself.
Afterwards, back at Orochimaru's lair, it is made apparent that Orochimaru plans to team up with the militaristic Konoha leader Danzo and destroy Konoha as it is today (the wording would seem to indicate a revolution or takeover, rather than outright annihilation). After a training exercise with Sasuke he interrupts Sai and Naruto, after they form a bond, to question Sai's loyalty. Though it seems like Orochimaru will resume his heated fight with Naruto at this point, he instead retreats, saying that he'll let Naruto go in the hopes that Naruto and company will take down more Akatsuki members for him. When Sasuke attempts to kill his former team with a new technique, Orochimaru and Kabuto appear and convinced him to spare their lives, at least until they kill more members of the Akatsuki. With Sasuke's "approval", they escape.
Defeat
While their training continued, Orochimaru watched as Sasuke defeated a large army of ninja alone, and remarked that Sasuke is much stronger than he was at his age, and slowly began to lose health. Sasuke saw this as an opportunity to leave Orochimaru as he was no longer strong enough to deserve his body, and attacked him while he was bedridden. Orochimaru reveals his true body, a large white snake made of several small snakes. However Sasuke activated his Cursed Seal and destroyed the giant snakes body.
Since his defeat, Orochimaru was suppressed by Sasuke's chakra. During his fight with Itachi, though, he uses up almost all of his chakra, and Orochimaru forces his way out of Sasuke. However, before he is able to defeat Itachi and then take Sasuke's body, Itachi uses the Totsuka Sword of his Susanoo to seal Orochimaru away, removing Sasuke's Cursed Seal. When Kabuto meets Naruto, Hinata Hyuga, and Yamato, he tells them how he infused himself with Orochimaru's remains, which are now slowly taking over his body, allowing Kabuto to take his power and finish Orochimaru's goals as a leader and not a follower.
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